FROM MOLECULES TO MATERIALS: UNDERSTANDING HYDROGEN ACTIVATION AND TRANSFER IN METAL OXIDES

Ref.No: 62430100
Start date: 25.11.2024
End date: 31.08.2026
Approval date: 06.11.2024
Department: CHEMICAL ENGINEERING
Sector: MATERIALS SCIENCE AND ENGINEERING
Financier: UNIVERSITY OF PITTSBURGH
Budget: 220.097,21 €
Public key: 9ΓΤΗ46ΨΖΣ4-63Κ
Scientific Responsible: Prof. IOANNIS MPOURMPAKIS
Email: gmpourmp@chemeng.ntua.gr
Description: THE RESEARCHERS AT NTUA WILL INVESTIGATE THE HYDROGEN EVOLUTION REACTION ON ANHYDROUS AND HYDRATED TUNGSTEN OXIDES HXWO3•2H2O, HXWO3•H2O AND HXWO3 AT PROTON COMPOSITION (DEGREE OF INTERCALATION), X LARGER THAN 0.5. THEY WILL USE DENSITY FUNCTIONAL THEORY (DFT) TO CALCULATE THE WATER-MEDIATED (HEYROVSKY) MECHANISM OF H2 FORMATION ON THE SURFACE OF THE CATALYSTS. IN ADDITION, SELECT CATALYSTS WILL BE DOPED WITH THE HETEROMETAL MO (GRADUAL REPLACEMENT OF W WITH MO) TO INVESTIGATE THE STABILITY OF THE MIXED OXIDE, THE THERMODYNAMICS OF PROTON INSERTION, AS WELL AS THE OXYGEN VACANCY FORMATION ENERGETICS.
ADDITIONALLY, POLYOXOMETALATE (POM) CLUSTERS WILL BE BROUGHT TOGETHER IN A SUPERCELL TO INVESTIGATE THE INTRAMOLECULAR BOND BREAKING AND INTERMOLECULAR BOND FORMING EVENTS, AT ELEVATED TEMPERATURES USING AB-INITIO MOLECULAR DYNAMICS.
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